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Polyaromatic Hydrocarbon (PAH) Pollution in Different Soil Uses: Spring Season

Year 2019, Volume: 21 Issue: 63, 805 - 817, 20.09.2019

Gizem Eker Şanlı Sabriye Sivri

https://doi.org/10.21205/deufmd.2019216311

Abstract



In
this study, the concentration and species distribution of polycyclic aromatic
hydrocarbons (PAHs) in the soils of olive groves in 7 different regions of
Bursa were investigated and toxicity risk assessments were performed. Soil
samples extracted by ultrasonic method and PAH concentrations were measured
by GC-MS. PAH pollution has been shown to have a large regional release
(2-2452 ng / g KM). The regions with the least and highest ∑12 PAH pollution
in the soils are the Mudanya Yörükali (MY) and Gemlik Campus (GK) regions
that their concentrations are measured as 2 ng / g KM and 2452 ng / g KM,
respectively. It is concluded that GK and MK are exposed to high PAH
contamination due to the regions where industrial, residential and
traffic-intensive regions are located. The low level of PAH contamination in
the MY region is thought to be due to the fact that this region is a rural
area away from pollutant sources. According to the regions, the distribution
of the ring was evaluated as 3 rings, 4 people and 5-6 rings. 87.3% of PAHs
in GK region consisted of 4 rings. In general, 4-ring PAH species were
dominant in sampling regions. The ∑12 BAPeq value ranges from 0.2 to 149.4 ng
/ g KM and the highest value is measured in the GK region. Risk assessment
was performed for PADs. ∑7 PAH cancer risk (CR) for GK region was measured in
the range of 3.39E-04-159E-0.3. 
Non-carcinogenic risk hazard coefficient (HQ) has been observed that
changed in the 0-0.14 range. It has been determined that PAH pollution has a
large regional release.

Keywords

Polycyclic Aromatic Hydrocarbons Soil Pollution PAHs Ring Distributions Toxicity Risk Assessments

References

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Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi

Year 2019, Volume: 21 Issue: 63, 805 - 817, 20.09.2019

Gizem Eker Şanlı Sabriye Sivri

https://doi.org/10.21205/deufmd.2019216311

Abstract

Bu çalışmada, Bursa’nın 7 farklı bölgesinde yer alan
zeytinlik arazilerinde topraklardaki polisiklik aromatik hidrokarbonların
(PAH’ların) konsantrasyonları, tür dağılımları incelenmiş ve toksisite risk
değerlendirmeleri yapılmıştır. Önemli bir sanayi ve tarım kenti olan Bursa’da
zeytinlik arazi topraklarında PAH kirlilik seviyesinin bölgesel değişiminin
ortaya konması amaçlanmıştır. Toprak örnekleri ultrasonik yöntemle ekstrakte edilmiş
ve PAH konsantrasyonları GC-MS ile ölçülmüştür. PAH kirliliğinin bölgesel
olarak büyük bir salınım gösterdiği tespit edilmiştir (2-2452 ng/g KM).
Topraklardaki ∑12 PAH kirliliğinin en az ve en fazla olduğu bölgeler sırasıyla
Mudanya Yörükali (MY) ve Gemlik Kampüs (GK) bölgeleri olup konsantrasyonları 2
ng/g KM ve 2452 ng/g KM olarak ölçülmüştür. GK ve MK, bölgelerinin sanayi,
yerleşim ve trafiğin yoğun olduğu bölgeler olması sebebiyle yüksek PAH
kirlenmesine maruz kaldığı sonucuna varılmıştır. MY bölgesinde PAH kirliliğinin
çok düşük seviyede olmasının, bu bölgenin kirletici kaynaklardan uzak ve kırsal
bir bölge olmasından kaynaklandığı düşünülmektedir. Bölgelere göre halka
dağılımları 3 halkalılar, 4halkalılar ve 5-6 halkalılar olarak
değerlendirilmiştir. GK bölgesinde PAH’ların % 87,3’ü 4 halkalılardan oluşmuştur.
Genel olarak örnekleme bölgelerinde 4 halkalı PAH türlerinin baskın olduğu
görülmüştür. ∑12 BAPeq  değeri 0,2- 149,4
ng/g KM arasında değişmekte olup en yüksek değer GK bölgesinde ölçülmüştür.
PAH’lar için risk değerlendirmesi yapılmıştır. GK bölgesi için ∑7 PAH kanser
risk (CR) değeri 3,39E-04-159E-0,3 aralığında ölçülmüştür. Kanserojen olmayan
risk tehlike katsayısı (HQ) 0-0,14 aralığında değiştiği gözlenmiştir.  PAH kirliliğinin bölgesel olarak büyük bir
salınım gösterdiği tespit edilmiştir.

Keywords

PAH Toprak kirliliği PAH halka dağılımları Toksisite ve Risk Değerlendirmeleri

References

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  • [20] Bozlaker, A., Muezzinoglu, A., & Odabasi, M. 2008. Atmospheric Concentrations, Dry Deposition and Air-Soil Exchange of Polycyclic Aromatic Hydrocarbons (PAHs) in An Industrial Region in Turkey. Journal of Hazardous Material, Cilt. 153, s.1093–1102. DOI:10.1016 /j.jhazmat.2007.09.064
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  • [22] Orecciho, S. 2010. Contamination from Polycyclic Aromatic Hydrocarbons (PAHs) in the Soil of a Botanic Garden Localized Next to a Former Manufacturing Gas Plant, Journal of Hazardous Materials, Cilt.15, s.590-601, doi:10.1016/j.jhazmat.2010.04.074.
  • [23] Wang, Y., Tian., Zhu, H., Cheng, Z., Kang, M. Luo, C.,Li, J., Zhang, G. 2012. Polycyclic Aromatic Hydrocarbons (PAHs) in Soils and Vegetation Near An E-Waste Recycling Site in South China: Concentration, Distribution, Source, and Risk Assessment. Science of the Total Environment, Cilt.439, s.187–193, https://doi.org/10.1016/j.scitotenv.2012.08.018
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  • [27] Choi, S.D. 2014. Time Trends in the Levels and Patterns of Polycyclic Aromatic Hydrocarbons (PAHs) İn Pine Bark, Litter, and Soil After A Forest Fire. Science of the Total Environment,Cilt.470,s.1441-1449.DOI:10.1016 /j.scitotenv. 2013.07.100
  • [28] Yang, Y., Zhang, X.X., Korenaga, T. 2002. Distribution of Polynuclear Aromatic Hydrocarbons (PAHs) in the Soil of Tokushima, Japan. Water Air Soil Pollution, Cilt.138, s.51-60. doi:Doi 10.1023/A:1015517504636
  • [29] Nadal, M., Schuhmacher, M., Domingo, J.L. 2004. Levels of PAHs in Soil and Vegetation Samples from Tarragona County, Spain. Environmental Pollution, Cilt.132, s.1-11. doi:DOI 10.1016/j.envpol.2004.04.003
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There are 40 citations in total.

Details

Primary Language Turkish
Subjects Engineering
Journal Section Articles
Authors

Gizem Eker Şanlı 0000-0002-7175-2942

Sabriye Sivri This is me 0000-0003-3472-6806

Publication Date September 20, 2019
Published in Issue Year 2019 Volume: 21 Issue: 63

Cite

APA Eker Şanlı, G., & Sivri, S. (2019). Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi. Dokuz Eylül Üniversitesi Mühendislik Fakültesi Fen Ve Mühendislik Dergisi, 21(63), 805-817. https://doi.org/10.21205/deufmd.2019216311
AMA Eker Şanlı G, Sivri S. Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi. DEUFMD. September 2019;21(63):805-817. doi:10.21205/deufmd.2019216311
Chicago Eker Şanlı, Gizem, and Sabriye Sivri. “Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi”. Dokuz Eylül Üniversitesi Mühendislik Fakültesi Fen Ve Mühendislik Dergisi 21, no. 63 (September 2019): 805-17. https://doi.org/10.21205/deufmd.2019216311.
EndNote Eker Şanlı G, Sivri S (September 1, 2019) Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi. Dokuz Eylül Üniversitesi Mühendislik Fakültesi Fen ve Mühendislik Dergisi 21 63 805–817.
IEEE G. Eker Şanlı and S. Sivri, “Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi”, DEUFMD, vol. 21, no. 63, pp. 805–817, 2019, doi: 10.21205/deufmd.2019216311.
ISNAD Eker Şanlı, Gizem - Sivri, Sabriye. “Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi”. Dokuz Eylül Üniversitesi Mühendislik Fakültesi Fen ve Mühendislik Dergisi 21/63 (September 2019), 805-817. https://doi.org/10.21205/deufmd.2019216311.
JAMA Eker Şanlı G, Sivri S. Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi. DEUFMD. 2019;21:805–817.
MLA Eker Şanlı, Gizem and Sabriye Sivri. “Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi”. Dokuz Eylül Üniversitesi Mühendislik Fakültesi Fen Ve Mühendislik Dergisi, vol. 21, no. 63, 2019, pp. 805-17, doi:10.21205/deufmd.2019216311.
Vancouver Eker Şanlı G, Sivri S. Farklı Toprak Kullanım Alanlarında Poliaromatik Hidrokarbon (PAH) Kirliliği: İlkbahar Mevsimi. DEUFMD. 2019;21(63):805-17.

Dokuz Eylül Üniversitesi, Mühendislik Fakültesi Dekanlığı Tınaztepe Yerleşkesi, Adatepe Mah. Doğuş Cad. No: 207-I / 35390 Buca-İZMİR.